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Dynamic anomalies at the glass transition of organic van der Waals liquids

The paper discusses the question of whether there is a characteristic temperature T"c above the calorimetric glass transition temperature T"g. Mode-coupling theory (MCT) predicts a crossover from liquid- to solid-like dynamics at T"c. Neutron scattering and gradient NMR experiments have been carried... Full description

Contributors: Fujara, F.
Sekundärausgabe Online edition, Elsevier Journal Backfiles on ScienceDirect 1907 - 2002 ; 041023-8
Contained in: Journal of Molecular Structure Amsterdam : Elsevier Vol. 296, No. 3 (1993), p. 285-294
Journal Title: Journal of Molecular Structure
Fulltext access: Fulltext access (direct link*)
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Links: Additional Link (linkinghub.elsevier.com)
ISSN: 0022-2860
Language: English
Notes: Copyright: Copyright (c) 2002 Elsevier Science B.V.
Physical Description: Online-Ressource
ID (e.g. DOI, URN): 0022-2860(93)80145-L
PPN (Catalogue-ID): NLEJ174409931
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520 |a The paper discusses the question of whether there is a characteristic temperature T"c above the calorimetric glass transition temperature T"g. Mode-coupling theory (MCT) predicts a crossover from liquid- to solid-like dynamics at T"c. Neutron scattering and gradient NMR experiments have been carried out to test MCT using the molecular van der Waals liquid ortho-terphenyl as a model system. A significant anomaly of the Debye-Waller factor and a ''decoupling'' of self-diffusion from viscosity support the MCT predictions. A critical discussion of the relevance of such tests and of the limitations of neutron scattering is presented. 
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