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Luminescence in Organic Silicons Prepared from Organic Precursors in Plasma Discharges

 The photoluminescence of plasma-prepared polysilanes during the change from linear 1D Si chains to an amorphous 3D Si network was studied. The excitonic absorption band with a maximum at 353 nm in 1D Si experiences a blue shift and broadening upon introduction of branching and networking defects. W... Full description

Main Author: Horváth, Pavel
Contributors: Schauer, František | Author
Kuřitka, Ivo | Author
Salyk, Ota | Author
Weiter, Martin | Author
Dokoupil, Norbert | Author
Nešpůrek, Stanislav | Author
Fidler, Vlastimil | Author
Contained in: Monatshefte für Chemie - Chemical Monthly : An International Journal of Chemistry Wien [u.a.] : Springer Vol. 132, No. 1 (2001), p. 177-183
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Links: Volltext (dx.doi.org)
ISSN: 1434-4475
Additional Keywords: Keywords. Silicon polymers; Plasma polymers; Luminescence; Effusion.
OriginalPaper
DOI: 10.1007/s007060170157
Language: English
Notes: Received July 10, 2000. Accepted (revised) September 8, 2000
Physical Description: Online-Ressource
ID (e.g. DOI, URN): 10.1007/s007060170157
s007060170157
PPN (Catalogue-ID): SPR019903650
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500 |a Received July 10, 2000. Accepted (revised) September 8, 2000 
520 |a  The photoluminescence of plasma-prepared polysilanes during the change from linear 1D Si chains to an amorphous 3D Si network was studied. The excitonic absorption band with a maximum at 353 nm in 1D Si experiences a blue shift and broadening upon introduction of branching and networking defects. With the gradual transition from 1D to 3D structure, an extensive redistribution of oscillator intensity along the absorption edge, accompanied by a decrease of the resolution of the σ-σ* band, was observed. In the short wavelength region of the excitation spectra there is an enormous increase of excitonic emission at 328 nm. This effect is tentatively attributed to the excitation of the phenyl group or to the phenyl-silicon bond as confirmed by effusion spectra of the phenyl species. 
653 |a OriginalPaper 
653 |a Keywords. Silicon polymers; Plasma polymers; Luminescence; Effusion. 
700 1 |a Schauer, František  |e verfasserin  |4 aut 
700 1 |a Kuřitka, Ivo  |e verfasserin  |4 aut 
700 1 |a Salyk, Ota  |e verfasserin  |4 aut 
700 1 |a Weiter, Martin  |e verfasserin  |4 aut 
700 1 |a Dokoupil, Norbert  |e verfasserin  |4 aut 
700 1 |a Nešpůrek, Stanislav  |e verfasserin  |4 aut 
700 1 |a Fidler, Vlastimil  |e verfasserin  |4 aut 
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